The influence of three important para- meters which affect the induration of iron-ore pellets, viz temperature, time, and lime content, have been assessed in terms of internal pellet structure and commonly-used pellet quality criteria. The pellets studied were produced from a typical hematite ore from the Pilbara area of Western Australia, using a 25 cm dia._x000D_
pot-grate test rig. Isothermal laboratory induration tests were conducted in accordance with a statistically-planned programme. The internal structures were studied by optical microscopic examination of polished sections of the test pellets. The effects of SFCA (silico- ferrite of calcium and aluminium) and slag formation, matrix consolidation and grain modi- fications were studied, and have been related to pellet properties and to the time/temperature histories produced by the firing conditions chosen. The implications of the data for commercial pellet plant operations are discussed.