Alumina reduction in Rajhara iron ore slimes essentially involves separation of hematite from gibbsite in relatively coarser fraction and from kaolinite in the finer fraction. Selective dispersion flocculation studies on synthetic mixtures clearly indicated that while it was possible to achieve almost perfect separation of hematite from kaolinite using starch and PAMX (modified polyacrylamide containing hydroxamate functional groups) flocculants, no selectivity was observed in iron oxide-alumina system. A schematic flowsheet suggested on the basis of this work for the beneficiation of Indian ore slimes thus consists of classification in a hydrocyclone, followed by selective dispersion of coarse fraction (underflow) and selective flocculation of the overflow fraction. Starting with a feed assaying 46 per cent Fe and 11.6 per cent A1203, a concentrate assaying 60 per cent Fe and 4.7 per cent A1203 could be produced at an overall iron recovery of 60 per cent using conventional Reagents.